TY - JOUR
T1 - CO2 electroreduction to ethylene via hydroxide-mediated copper catalysis at an abrupt interface
AU - Dinh, Cao Thang
AU - Burdyny, Thomas
AU - Kibria, Golam
AU - Seifitokaldani, Ali
AU - Gabardo, Christine M.
AU - Pelayo García De Arquer, F.
AU - Kiani, Amirreza
AU - Edwards, Jonathan P.
AU - De Luna, Phil
AU - Bushuyev, Oleksandr S.
AU - Zou, Chengqin
AU - Quintero-Bermudez, Rafael
AU - Pang, Yuanjie
AU - Sinton, David
AU - Sargent, Edward H.
N1 - Publisher Copyright:
© 2018 American Association for the Advancement of Science. All rights reserved.
PY - 2018/5/18
Y1 - 2018/5/18
N2 - Carbon dioxide (CO2) electroreduction could provide a useful source of ethylene, but low conversion efficiency, low production rates, and low catalyst stability limit current systems. Here we report that a copper electrocatalyst at an abrupt reaction interface in an alkaline electrolyte reduces CO2 to ethylene with 70% faradaic efficiency at a potential of -0.55 volts versus a reversible hydrogen electrode (RHE). Hydroxide ions on or near the copper surface lower the CO2 reduction and carbon monoxide (CO)-CO coupling activation energy barriers; as a result, onset of ethylene evolution at -0.165 volts versus an RHE in 10 molar potassium hydroxide occurs almost simultaneously with CO production. Operational stability was enhanced via the introduction of a polymer-based gas diffusion layer that sandwiches the reaction interface between separate hydrophobic and conductive supports, providing constant ethylene selectivity for an initial 150 operating hours.
AB - Carbon dioxide (CO2) electroreduction could provide a useful source of ethylene, but low conversion efficiency, low production rates, and low catalyst stability limit current systems. Here we report that a copper electrocatalyst at an abrupt reaction interface in an alkaline electrolyte reduces CO2 to ethylene with 70% faradaic efficiency at a potential of -0.55 volts versus a reversible hydrogen electrode (RHE). Hydroxide ions on or near the copper surface lower the CO2 reduction and carbon monoxide (CO)-CO coupling activation energy barriers; as a result, onset of ethylene evolution at -0.165 volts versus an RHE in 10 molar potassium hydroxide occurs almost simultaneously with CO production. Operational stability was enhanced via the introduction of a polymer-based gas diffusion layer that sandwiches the reaction interface between separate hydrophobic and conductive supports, providing constant ethylene selectivity for an initial 150 operating hours.
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U2 - 10.1126/science.aas9100
DO - 10.1126/science.aas9100
M3 - Article
C2 - 29773749
AN - SCOPUS:85047563747
SN - 0036-8075
VL - 360
SP - 783
EP - 787
JO - Science
JF - Science
IS - 6390
ER -