Discovery Principles and Materials for Symmetry-Protected Persistent Spin Textures with Long Spin Lifetimes

Xue Zeng Lu; James M. Rondinelli

doi:10.1016/j.matt.2020.08.028

Discovery Principles and Materials for Symmetry-Protected Persistent Spin Textures with Long Spin Lifetimes

Xue Zeng Lu, James M. Rondinelli^*

^*Corresponding author for this work

Materials Science and Engineering

Research output: Contribution to journal › Article › peer-review

1 Scopus citations

Abstract

To design materials possessing high-quality persistent spin textures (PSTs), both the spin lifetime (τ_s) and portion of the Brillouin zone exhibiting the PST (S) require optimization. We find τ_s and S are optimal with moderate spin-orbit coupling (SOC) parameters. Furthermore, τ_s and S can be tuned by the magnitude of the BX₆ octahedral rotations in perovskite-derived materials, which governs the PST in a manner opposite to that from intrinsic SOC (Δ_SOC), enabling discovery of optimal PST materials with strong SOC.

Original language	English (US)
Pages (from-to)	1211-1225
Number of pages	15
Journal	Matter
Volume	3
Issue number	4
DOIs	https://doi.org/10.1016/j.matt.2020.08.028
State	Published - Oct 7 2020

Keywords

MAP1: Discovery

ASJC Scopus subject areas

Materials Science(all)

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@article{c492439f2d2e4b058987adcc74165bf4,

title = "Discovery Principles and Materials for Symmetry-Protected Persistent Spin Textures with Long Spin Lifetimes",

abstract = "To design materials possessing high-quality persistent spin textures (PSTs), both the spin lifetime (τs) and portion of the Brillouin zone exhibiting the PST (S) require optimization. We find τs and S are optimal with moderate spin-orbit coupling (SOC) parameters. Furthermore, τs and S can be tuned by the magnitude of the BX6 octahedral rotations in perovskite-derived materials, which governs the PST in a manner opposite to that from intrinsic SOC (ΔSOC), enabling discovery of optimal PST materials with strong SOC.",

keywords = "MAP1: Discovery",

author = "Lu, {Xue Zeng} and Rondinelli, {James M.}",

note = "Funding Information: X.-Z.L. and J.M.R. were supported by the Army Research Office under grant no. W911NF-15-1-0017 . DFT calculations were performed on the CARBON cluster at the Center for Nanoscale Materials at Argonne National Laboratory and the Extreme Science and Engineering Discovery Environment, which is supported by NSF ( ACI-1548562 ). Use of the Center for Nanoscale Materials, an Office of Science user facility, was supported by the US Department of Energy , Office of Science , Office of Basic Energy Sciences , under contract no. DE-AC02-06CH11357. ",

year = "2020",

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doi = "10.1016/j.matt.2020.08.028",

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AU - Lu, Xue Zeng

AU - Rondinelli, James M.

N1 - Funding Information: X.-Z.L. and J.M.R. were supported by the Army Research Office under grant no. W911NF-15-1-0017 . DFT calculations were performed on the CARBON cluster at the Center for Nanoscale Materials at Argonne National Laboratory and the Extreme Science and Engineering Discovery Environment, which is supported by NSF ( ACI-1548562 ). Use of the Center for Nanoscale Materials, an Office of Science user facility, was supported by the US Department of Energy , Office of Science , Office of Basic Energy Sciences , under contract no. DE-AC02-06CH11357.

PY - 2020/10/7

Y1 - 2020/10/7

N2 - To design materials possessing high-quality persistent spin textures (PSTs), both the spin lifetime (τs) and portion of the Brillouin zone exhibiting the PST (S) require optimization. We find τs and S are optimal with moderate spin-orbit coupling (SOC) parameters. Furthermore, τs and S can be tuned by the magnitude of the BX6 octahedral rotations in perovskite-derived materials, which governs the PST in a manner opposite to that from intrinsic SOC (ΔSOC), enabling discovery of optimal PST materials with strong SOC.

AB - To design materials possessing high-quality persistent spin textures (PSTs), both the spin lifetime (τs) and portion of the Brillouin zone exhibiting the PST (S) require optimization. We find τs and S are optimal with moderate spin-orbit coupling (SOC) parameters. Furthermore, τs and S can be tuned by the magnitude of the BX6 octahedral rotations in perovskite-derived materials, which governs the PST in a manner opposite to that from intrinsic SOC (ΔSOC), enabling discovery of optimal PST materials with strong SOC.

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