Abstract
The TDSCF approximation is applied to dissociation of Ar3, which exhibits strong-coupling behavior (efficient internal energy transfer). The TDSCF results are in excellent agreement with those of exact classical dynamics. Combined with earlier findings for weak-coupling cases, this suggests validity of TDSCF for dissociation at all coupling strengths.
Original language | English (US) |
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Pages (from-to) | 44-48 |
Number of pages | 5 |
Journal | Chemical Physics Letters |
Volume | 101 |
Issue number | 1 |
DOIs | |
State | Published - Oct 7 1983 |
Funding
The Fritz Haber Center is supported by the Minerva Ceselschaft fiir die Forschung mbH, Munich, FRG.
ASJC Scopus subject areas
- General Physics and Astronomy
- Physical and Theoretical Chemistry