Electron hopping among cofacially stacked perylenediimides assembled by using DNA hairpins

Thea M. Wilson; Torek A. Zeidan; Mahesh Hariharan; Frederick D. Lewis; Michael R. Wasielewski

doi:10.1002/anie.200907339

Electron hopping among cofacially stacked perylenediimides assembled by using DNA hairpins

Thea M. Wilson, Torek A. Zeidan, Mahesh Hariharan, Frederick D. Lewis, Michael R. Wasielewski

Chemistry

Research output: Contribution to journal › Article › peer-review

61 Scopus citations

Abstract

(Figure Presented) Charge on through: Perylenediimide chromophores incorporated into DNA hairpins serve as base-pair surrogates and form a zipperlike intercalated structure (see picture). Electron hopping was observed within the chromophore stacks upon one-electron reduction.

Original language	English (US)
Pages (from-to)	2385-2388
Number of pages	4
Journal	Angewandte Chemie - International Edition
Volume	49
Issue number	13
DOIs	https://doi.org/10.1002/anie.200907339
State	Published - Mar 22 2010

Keywords

Chromophores
DNA
ENDOR spectroscopy
EPR spectroscopy
Electron transport

ASJC Scopus subject areas

General Chemistry
Catalysis

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10.1002/anie.200907339

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title = "Electron hopping among cofacially stacked perylenediimides assembled by using DNA hairpins",

abstract = "(Figure Presented) Charge on through: Perylenediimide chromophores incorporated into DNA hairpins serve as base-pair surrogates and form a zipperlike intercalated structure (see picture). Electron hopping was observed within the chromophore stacks upon one-electron reduction.",

keywords = "Chromophores, DNA, ENDOR spectroscopy, EPR spectroscopy, Electron transport",

author = "Wilson, {Thea M.} and Zeidan, {Torek A.} and Mahesh Hariharan and Lewis, {Frederick D.} and Wasielewski, {Michael R.}",

year = "2010",

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AU - Zeidan, Torek A.

AU - Hariharan, Mahesh

AU - Lewis, Frederick D.

AU - Wasielewski, Michael R.

PY - 2010/3/22

Y1 - 2010/3/22

N2 - (Figure Presented) Charge on through: Perylenediimide chromophores incorporated into DNA hairpins serve as base-pair surrogates and form a zipperlike intercalated structure (see picture). Electron hopping was observed within the chromophore stacks upon one-electron reduction.

AB - (Figure Presented) Charge on through: Perylenediimide chromophores incorporated into DNA hairpins serve as base-pair surrogates and form a zipperlike intercalated structure (see picture). Electron hopping was observed within the chromophore stacks upon one-electron reduction.

KW - Chromophores

KW - DNA

KW - ENDOR spectroscopy

KW - EPR spectroscopy

KW - Electron transport

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Electron hopping among cofacially stacked perylenediimides assembled by using DNA hairpins

Abstract

Keywords

ASJC Scopus subject areas

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