TY - JOUR
T1 - Electronic Transport in Two-Dimensional Materials
AU - Sangwan, Vinod K.
AU - Hersam, Mark C.
N1 - Funding Information:
The authors acknowledge support from the National Science Foundation Materials Research Science and Engineering Center (DMR-1720139) and 2-DARE program (EFRI-1433510).
Publisher Copyright:
© 2018 by Annual Reviews. All rights reserved.
PY - 2018/4/20
Y1 - 2018/4/20
N2 - Two-dimensional (2D) materials have captured the attention of the scientific community due to the wide range of unique properties at nanometer-scale thicknesses. While significant exploratory research in 2D materials has been achieved, the understanding of 2D electronic transport and carrier dynamics remains in a nascent stage. Furthermore, because prior review articles have provided general overviews of 2D materials or specifically focused on charge transport in graphene, here we instead highlight charge transport mechanisms in post-graphene 2D materials, with particular emphasis on transition metal dichalcogenides and black phosphorus. For these systems, we delineate the intricacies of electronic transport, including band structure control with thickness and external fields, valley polarization, scattering mechanisms, electrical contacts, and doping. In addition, electronic interactions between 2D materials are considered in the form of van der Waals heterojunctions and composite films. This review concludes with a perspective on the most promising future directions in this fast-evolving field.
AB - Two-dimensional (2D) materials have captured the attention of the scientific community due to the wide range of unique properties at nanometer-scale thicknesses. While significant exploratory research in 2D materials has been achieved, the understanding of 2D electronic transport and carrier dynamics remains in a nascent stage. Furthermore, because prior review articles have provided general overviews of 2D materials or specifically focused on charge transport in graphene, here we instead highlight charge transport mechanisms in post-graphene 2D materials, with particular emphasis on transition metal dichalcogenides and black phosphorus. For these systems, we delineate the intricacies of electronic transport, including band structure control with thickness and external fields, valley polarization, scattering mechanisms, electrical contacts, and doping. In addition, electronic interactions between 2D materials are considered in the form of van der Waals heterojunctions and composite films. This review concludes with a perspective on the most promising future directions in this fast-evolving field.
KW - Black phosphorus
KW - Contacts
KW - Doping
KW - Scattering
KW - Transition metal dichalcogenide
KW - Van der Waals heterojunction
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U2 - 10.1146/annurev-physchem-050317-021353
DO - 10.1146/annurev-physchem-050317-021353
M3 - Article
C2 - 29463170
AN - SCOPUS:85045879144
SN - 0066-426X
VL - 69
SP - 299
EP - 325
JO - Annual Review of Physical Chemistry
JF - Annual Review of Physical Chemistry
ER -