Fourier transform two-dimensional electronic-vibrational spectroscopy using an octave-spanning mid-IR probe

James D. Gaynor, Trevor L. Courtney, Madhumitha Balasubramanian, Munira Khalil*

*Corresponding author for this work

Research output: Contribution to journalArticlepeer-review

42 Scopus citations

Abstract

The development of coherent Fourier transform two-dimensional electronic-vibrational (2D EV) spectroscopy with acousto-optic pulse-shaper-generated near-UV pump pulses and an octave-spanning broadband mid-IR probe pulse is detailed. A 2D EV spectrum of a silicon wafer demonstrates the full experimental capability of this experiment, and a 2D EV spectrum of dissolved hexacyanoferrate establishes the viability of our 2D EV experiment for studying condensed phase molecular ensembles.

Original languageEnglish (US)
Pages (from-to)2895-2898
Number of pages4
JournalOptics Letters
Volume41
Issue number12
DOIs
StatePublished - Jun 15 2016

ASJC Scopus subject areas

  • Atomic and Molecular Physics, and Optics

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