Granular mixtures: Analogy with chemical solution thermodynamics

B. L. Severson*, R. Q. Snurr, J. M. Ottino

*Corresponding author for this work

Research output: Contribution to journalArticlepeer-review

3 Scopus citations

Abstract

Particle dynamics simulations reveal parallels between granular mixtures and chemical solutions. Thermodynamic solution theory provides a connection between the interaction strength of the molecules, the concentration of each species in the solution, and bulk solution behavior. Particle dynamics simulations demonstrate a similar relationship between the interparticle forces, the composition of the granular mixture, and bulk flow behavior. The analogy holds true over different particle interaction types (friction or adhesion) and over different bulk properties (the angle of repose in a rotating drum and the viscosity of particles sheared between parallel plates). A solution theory for granular mixtures would provide a framework to study the properties of granular mixtures.

Original languageEnglish (US)
Article number174902
JournalJournal of Chemical Physics
Volume127
Issue number17
DOIs
StatePublished - 2007

Funding

The authors thank the U.S. National Science Foundation IGERT program and the Air Force Office of Scientific Research for funding.

ASJC Scopus subject areas

  • General Physics and Astronomy
  • Physical and Theoretical Chemistry

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