Hyper-Rayleigh scattering from silver nanoparticles

E. C. Hao; G. C. Schatz; R. C. Johnson; J. T. Hupp

doi:10.1063/1.1510439

Hyper-Rayleigh scattering from silver nanoparticles

E. C. Hao, G. C. Schatz^*, R. C. Johnson, J. T. Hupp

^*Corresponding author for this work

Chemistry

Research output: Contribution to journal › Article › peer-review

136 Scopus citations

Abstract

A study was conducted on the leading-order contribution to the incoherent second harmonic generation of silver nanoparticles. By measuring the excitation wavelength dependence of β_silver, distinguishable dipole and quadrupole plasmon contributions to hyper-Rayleigh intensities were experimentally demonstrated. These two contributions have different angular distributions, and it was shown that DSEH theory in conjunction with simple angular distribution measurements may be used to determine the relative sizes of the dipole and quadrupole contributions.

Original language	English (US)
Pages (from-to)	5963-5966
Number of pages	4
Journal	Journal of Chemical Physics
Volume	117
Issue number	13
DOIs	https://doi.org/10.1063/1.1510439
State	Published - Oct 1 2002

ASJC Scopus subject areas

General Physics and Astronomy
Physical and Theoretical Chemistry

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10.1063/1.1510439

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abstract = "A study was conducted on the leading-order contribution to the incoherent second harmonic generation of silver nanoparticles. By measuring the excitation wavelength dependence of βsilver, distinguishable dipole and quadrupole plasmon contributions to hyper-Rayleigh intensities were experimentally demonstrated. These two contributions have different angular distributions, and it was shown that DSEH theory in conjunction with simple angular distribution measurements may be used to determine the relative sizes of the dipole and quadrupole contributions.",

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N2 - A study was conducted on the leading-order contribution to the incoherent second harmonic generation of silver nanoparticles. By measuring the excitation wavelength dependence of βsilver, distinguishable dipole and quadrupole plasmon contributions to hyper-Rayleigh intensities were experimentally demonstrated. These two contributions have different angular distributions, and it was shown that DSEH theory in conjunction with simple angular distribution measurements may be used to determine the relative sizes of the dipole and quadrupole contributions.

AB - A study was conducted on the leading-order contribution to the incoherent second harmonic generation of silver nanoparticles. By measuring the excitation wavelength dependence of βsilver, distinguishable dipole and quadrupole plasmon contributions to hyper-Rayleigh intensities were experimentally demonstrated. These two contributions have different angular distributions, and it was shown that DSEH theory in conjunction with simple angular distribution measurements may be used to determine the relative sizes of the dipole and quadrupole contributions.

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Hyper-Rayleigh scattering from silver nanoparticles

Abstract

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