Investigation of volatile liquid surfaces by synchrotron x-ray spectroscopy of liquid microjets

Kevin R. Wilson; Bruce S. Rude; Jared Smith; Chris Cappa; D. T. Co; R. D. Schaller; M. Larsson; T. Catalano; R. J. Saykally

doi:10.1063/1.1645656

Investigation of volatile liquid surfaces by synchrotron x-ray spectroscopy of liquid microjets

Kevin R. Wilson, Bruce S. Rude, Jared Smith, Chris Cappa, D. T. Co, R. D. Schaller, M. Larsson, T. Catalano, R. J. Saykally^*

^*Corresponding author for this work

Chemistry

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113 Scopus citations

Abstract

The development of x-ray absorption spectroscopy (XAS) for the study of volatile liquid surfaces using microjets was discussed. The design and implementation of x-ray experiment based on the use of liquid microjets were described. The experiments characterizing the temperature of liquid water and methanol streams injected into high vacuum through microjet nozzles were analyzed. It was shown that the application of high-vacuum XAS techniques to liquid microjets allows a particular class of measurements to be performed on volatile liquid surfaces without significant interference from the equilibrium vapor.

Original language	English (US)
Pages (from-to)	725-736
Number of pages	12
Journal	Review of Scientific Instruments
Volume	75
Issue number	3
DOIs	https://doi.org/10.1063/1.1645656
State	Published - Mar 2004

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Instrumentation

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title = "Investigation of volatile liquid surfaces by synchrotron x-ray spectroscopy of liquid microjets",

abstract = "The development of x-ray absorption spectroscopy (XAS) for the study of volatile liquid surfaces using microjets was discussed. The design and implementation of x-ray experiment based on the use of liquid microjets were described. The experiments characterizing the temperature of liquid water and methanol streams injected into high vacuum through microjet nozzles were analyzed. It was shown that the application of high-vacuum XAS techniques to liquid microjets allows a particular class of measurements to be performed on volatile liquid surfaces without significant interference from the equilibrium vapor.",

author = "Wilson, {Kevin R.} and Rude, {Bruce S.} and Jared Smith and Chris Cappa and Co, {D. T.} and Schaller, {R. D.} and M. Larsson and T. Catalano and Saykally, {R. J.}",

year = "2004",

month = mar,

doi = "10.1063/1.1645656",

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AU - Wilson, Kevin R.

AU - Rude, Bruce S.

AU - Smith, Jared

AU - Cappa, Chris

AU - Co, D. T.

AU - Schaller, R. D.

AU - Larsson, M.

AU - Catalano, T.

AU - Saykally, R. J.

PY - 2004/3

Y1 - 2004/3

N2 - The development of x-ray absorption spectroscopy (XAS) for the study of volatile liquid surfaces using microjets was discussed. The design and implementation of x-ray experiment based on the use of liquid microjets were described. The experiments characterizing the temperature of liquid water and methanol streams injected into high vacuum through microjet nozzles were analyzed. It was shown that the application of high-vacuum XAS techniques to liquid microjets allows a particular class of measurements to be performed on volatile liquid surfaces without significant interference from the equilibrium vapor.

AB - The development of x-ray absorption spectroscopy (XAS) for the study of volatile liquid surfaces using microjets was discussed. The design and implementation of x-ray experiment based on the use of liquid microjets were described. The experiments characterizing the temperature of liquid water and methanol streams injected into high vacuum through microjet nozzles were analyzed. It was shown that the application of high-vacuum XAS techniques to liquid microjets allows a particular class of measurements to be performed on volatile liquid surfaces without significant interference from the equilibrium vapor.

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Investigation of volatile liquid surfaces by synchrotron x-ray spectroscopy of liquid microjets

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