Abstract
We introduce an optimal control approach that is capable of yielding the best achievable field-free three-dimensional (3-D) alignment in an arbitrary molecule. Our analysis provides the optimal route to the best aligned state along with interesting insights into the 3-D alignment dynamics of polyatomic systems.
| Original language | English (US) |
|---|---|
| Article number | 023413 |
| Journal | Physical Review A - Atomic, Molecular, and Optical Physics |
| Volume | 82 |
| Issue number | 2 |
| DOIs | |
| State | Published - Aug 12 2010 |
ASJC Scopus subject areas
- Atomic and Molecular Physics, and Optics