Polarized resonant Raman study of isolated single-wall carbon nanotubes: Symmetry selection rules, dipolar and multipolar antenna effects

A. Jorio; A. G. Souza Filho; A. G. Souza Filho; V. W. Brar; A. K. Swan; M. S. Ünlü; B. B. Goldberg; B. B. Goldberg; A. Righi; J. H. Hafner; C. M. Lieber; R. Saito; G. Dresselhaus; M. S. Dresselhaus; M. S. Dresselhaus

Polarized resonant Raman study of isolated single-wall carbon nanotubes: Symmetry selection rules, dipolar and multipolar antenna effects

A. Jorio, A. G. Souza Filho, A. G. Souza Filho, V. W. Brar, A. K. Swan, M. S. Ünlü, B. B. Goldberg, B. B. Goldberg, A. Righi, J. H. Hafner, C. M. Lieber, R. Saito, G. Dresselhaus, M. S. Dresselhaus, M. S. Dresselhaus

Physics and Astronomy

Research output: Contribution to journal › Article › peer-review

137 Scopus citations

Abstract

We studied the polarization dependence of the resonance Raman spectra for several different isolated singlewall carbon nanotubes (SWNTs). One isolated SWNT acts as a dipolar antenna, polarized along the tube axis. For light polarized parallel to the tube axis, the strong resonance-effect breaks the symmetry-selection rules, and symmetry-forbidden modes appear in the Raman spectrum. When the light is not polarized parallel to the tube axis, G-band mode symmetries can be identified. Unusual G-mode intensity behavior is observed when the Raman signal is obtained from more than one SWNT, suggesting a complex multipolar antenna pattern.

Original language	English (US)
Article number	121402
Pages (from-to)	1214021-1214024
Number of pages	4
Journal	Physical Review B - Condensed Matter and Materials Physics
Volume	65
Issue number	12
State	Published - Mar 15 2002

ASJC Scopus subject areas

Electronic, Optical and Magnetic Materials
Condensed Matter Physics

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Jorio, A., Souza Filho, A. G., Souza Filho, A. G., Brar, V. W., Swan, A. K., Ünlü, M. S., Goldberg, B. B., Goldberg, B. B., Righi, A., Hafner, J. H., Lieber, C. M., Saito, R., Dresselhaus, G., Dresselhaus, M. S., & Dresselhaus, M. S. (2002). Polarized resonant Raman study of isolated single-wall carbon nanotubes: Symmetry selection rules, dipolar and multipolar antenna effects. Physical Review B - Condensed Matter and Materials Physics, 65(12), 1214021-1214024. [121402].

Jorio, A. ; Souza Filho, A. G. ; Souza Filho, A. G. ; Brar, V. W. ; Swan, A. K. ; Ünlü, M. S. ; Goldberg, B. B. ; Goldberg, B. B. ; Righi, A. ; Hafner, J. H. ; Lieber, C. M. ; Saito, R. ; Dresselhaus, G. ; Dresselhaus, M. S. ; Dresselhaus, M. S. / Polarized resonant Raman study of isolated single-wall carbon nanotubes : Symmetry selection rules, dipolar and multipolar antenna effects. In: Physical Review B - Condensed Matter and Materials Physics. 2002 ; Vol. 65, No. 12. pp. 1214021-1214024.

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title = "Polarized resonant Raman study of isolated single-wall carbon nanotubes: Symmetry selection rules, dipolar and multipolar antenna effects",

abstract = "We studied the polarization dependence of the resonance Raman spectra for several different isolated singlewall carbon nanotubes (SWNTs). One isolated SWNT acts as a dipolar antenna, polarized along the tube axis. For light polarized parallel to the tube axis, the strong resonance-effect breaks the symmetry-selection rules, and symmetry-forbidden modes appear in the Raman spectrum. When the light is not polarized parallel to the tube axis, G-band mode symmetries can be identified. Unusual G-mode intensity behavior is observed when the Raman signal is obtained from more than one SWNT, suggesting a complex multipolar antenna pattern.",

author = "A. Jorio and {Souza Filho}, {A. G.} and {Souza Filho}, {A. G.} and Brar, {V. W.} and Swan, {A. K.} and {\"U}nl{\"u}, {M. S.} and Goldberg, {B. B.} and Goldberg, {B. B.} and A. Righi and Hafner, {J. H.} and Lieber, {C. M.} and R. Saito and G. Dresselhaus and Dresselhaus, {M. S.} and Dresselhaus, {M. S.}",

year = "2002",

month = mar,

day = "15",

language = "English (US)",

volume = "65",

pages = "1214021--1214024",

journal = "Physical Review B - Condensed Matter and Materials Physics",

issn = "1098-0121",

publisher = "American Physical Society",

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Jorio, A, Souza Filho, AG, Souza Filho, AG, Brar, VW, Swan, AK, Ünlü, MS, Goldberg, BB, Goldberg, BB, Righi, A, Hafner, JH, Lieber, CM, Saito, R, Dresselhaus, G, Dresselhaus, MS & Dresselhaus, MS 2002, 'Polarized resonant Raman study of isolated single-wall carbon nanotubes: Symmetry selection rules, dipolar and multipolar antenna effects', Physical Review B - Condensed Matter and Materials Physics, vol. 65, no. 12, 121402, pp. 1214021-1214024.

Polarized resonant Raman study of isolated single-wall carbon nanotubes : Symmetry selection rules, dipolar and multipolar antenna effects. / Jorio, A.; Souza Filho, A. G.; Souza Filho, A. G.; Brar, V. W.; Swan, A. K.; Ünlü, M. S.; Goldberg, B. B.; Goldberg, B. B.; Righi, A.; Hafner, J. H.; Lieber, C. M.; Saito, R.; Dresselhaus, G.; Dresselhaus, M. S.; Dresselhaus, M. S.

In: Physical Review B - Condensed Matter and Materials Physics, Vol. 65, No. 12, 121402, 15.03.2002, p. 1214021-1214024.

Research output: Contribution to journal › Article › peer-review

TY - JOUR

T1 - Polarized resonant Raman study of isolated single-wall carbon nanotubes

T2 - Symmetry selection rules, dipolar and multipolar antenna effects

AU - Jorio, A.

AU - Souza Filho, A. G.

AU - Brar, V. W.

AU - Swan, A. K.

AU - Ünlü, M. S.

AU - Goldberg, B. B.

AU - Righi, A.

AU - Hafner, J. H.

AU - Lieber, C. M.

AU - Saito, R.

AU - Dresselhaus, G.

AU - Dresselhaus, M. S.

PY - 2002/3/15

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N2 - We studied the polarization dependence of the resonance Raman spectra for several different isolated singlewall carbon nanotubes (SWNTs). One isolated SWNT acts as a dipolar antenna, polarized along the tube axis. For light polarized parallel to the tube axis, the strong resonance-effect breaks the symmetry-selection rules, and symmetry-forbidden modes appear in the Raman spectrum. When the light is not polarized parallel to the tube axis, G-band mode symmetries can be identified. Unusual G-mode intensity behavior is observed when the Raman signal is obtained from more than one SWNT, suggesting a complex multipolar antenna pattern.

AB - We studied the polarization dependence of the resonance Raman spectra for several different isolated singlewall carbon nanotubes (SWNTs). One isolated SWNT acts as a dipolar antenna, polarized along the tube axis. For light polarized parallel to the tube axis, the strong resonance-effect breaks the symmetry-selection rules, and symmetry-forbidden modes appear in the Raman spectrum. When the light is not polarized parallel to the tube axis, G-band mode symmetries can be identified. Unusual G-mode intensity behavior is observed when the Raman signal is obtained from more than one SWNT, suggesting a complex multipolar antenna pattern.

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ER -

Polarized resonant Raman study of isolated single-wall carbon nanotubes: Symmetry selection rules, dipolar and multipolar antenna effects

Abstract

ASJC Scopus subject areas

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