Prediction of new multiplet structure in photoemission experiments

P. S. Bagus; A. J. Freeman; F. Sasaki

doi:10.1103/PhysRevLett.30.850

Prediction of new multiplet structure in photoemission experiments

P. S. Bagus^*, A. J. Freeman, F. Sasaki

^*Corresponding author for this work

Physics and Astronomy

Research output: Contribution to journal › Article › peer-review

221 Scopus citations

Abstract

Correlation effects are included in a detailed theoretical study of the multiplet structure observed by x-ray photoelectron spectroscopy. This correlated multiplet hole theory resolves the difficulties of earlier multiplet hole theory studies: It correctly determines the magnitude of the observed 2s and 3s (doublet) splittings and their intensity rations, and predicts the existence of new structure for the 3s binding energy splittings-structure which does not exist in one-electron theory and which has now been confirmed by Kowalczyk et al.

Original language	English (US)
Pages (from-to)	850-853
Number of pages	4
Journal	Physical review letters
Volume	30
Issue number	18
DOIs	https://doi.org/10.1103/PhysRevLett.30.850
State	Published - 1973

ASJC Scopus subject areas

General Physics and Astronomy

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10.1103/PhysRevLett.30.850

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title = "Prediction of new multiplet structure in photoemission experiments",

abstract = "Correlation effects are included in a detailed theoretical study of the multiplet structure observed by x-ray photoelectron spectroscopy. This correlated multiplet hole theory resolves the difficulties of earlier multiplet hole theory studies: It correctly determines the magnitude of the observed 2s and 3s (doublet) splittings and their intensity rations, and predicts the existence of new structure for the 3s binding energy splittings-structure which does not exist in one-electron theory and which has now been confirmed by Kowalczyk et al.",

author = "Bagus, {P. S.} and Freeman, {A. J.} and F. Sasaki",

note = "Funding Information: Work supported by the U. S. Air Force Office of Scientific Research, by the U. S. Atomic Energy Commission, and by the National Science Foundation. Copyright: Copyright 2015 Elsevier B.V., All rights reserved.",

year = "1973",

doi = "10.1103/PhysRevLett.30.850",

language = "English (US)",

volume = "30",

pages = "850--853",

journal = "Physical review letters",

issn = "0031-9007",

publisher = "American Physical Society",

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T1 - Prediction of new multiplet structure in photoemission experiments

AU - Bagus, P. S.

AU - Freeman, A. J.

AU - Sasaki, F.

N1 - Funding Information: Work supported by the U. S. Air Force Office of Scientific Research, by the U. S. Atomic Energy Commission, and by the National Science Foundation. Copyright: Copyright 2015 Elsevier B.V., All rights reserved.

PY - 1973

Y1 - 1973

N2 - Correlation effects are included in a detailed theoretical study of the multiplet structure observed by x-ray photoelectron spectroscopy. This correlated multiplet hole theory resolves the difficulties of earlier multiplet hole theory studies: It correctly determines the magnitude of the observed 2s and 3s (doublet) splittings and their intensity rations, and predicts the existence of new structure for the 3s binding energy splittings-structure which does not exist in one-electron theory and which has now been confirmed by Kowalczyk et al.

AB - Correlation effects are included in a detailed theoretical study of the multiplet structure observed by x-ray photoelectron spectroscopy. This correlated multiplet hole theory resolves the difficulties of earlier multiplet hole theory studies: It correctly determines the magnitude of the observed 2s and 3s (doublet) splittings and their intensity rations, and predicts the existence of new structure for the 3s binding energy splittings-structure which does not exist in one-electron theory and which has now been confirmed by Kowalczyk et al.

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DO - 10.1103/PhysRevLett.30.850

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JO - Physical review letters

JF - Physical review letters

IS - 18

ER -

Prediction of new multiplet structure in photoemission experiments

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