Prediction of new multiplet structure in photoemission experiments

P. S. Bagus; A. J. Freeman; F. Sasaki

doi:10.1103/PhysRevLett.30.850

Prediction of new multiplet structure in photoemission experiments

P. S. Bagus^*, A. J. Freeman, F. Sasaki

^*Corresponding author for this work

Physics and Astronomy

Research output: Contribution to journal › Article › peer-review

222 Scopus citations

Abstract

Correlation effects are included in a detailed theoretical study of the multiplet structure observed by x-ray photoelectron spectroscopy. This correlated multiplet hole theory resolves the difficulties of earlier multiplet hole theory studies: It correctly determines the magnitude of the observed 2s and 3s (doublet) splittings and their intensity rations, and predicts the existence of new structure for the 3s binding energy splittings-structure which does not exist in one-electron theory and which has now been confirmed by Kowalczyk et al.

Original language	English (US)
Pages (from-to)	850-853
Number of pages	4
Journal	Physical review letters
Volume	30
Issue number	18
DOIs	https://doi.org/10.1103/PhysRevLett.30.850
State	Published - 1973

Funding

Work supported by the U. S. Air Force Office of Scientific Research, by the U. S. Atomic Energy Commission, and by the National Science Foundation.

ASJC Scopus subject areas

General Physics and Astronomy

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10.1103/PhysRevLett.30.850

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title = "Prediction of new multiplet structure in photoemission experiments",

abstract = "Correlation effects are included in a detailed theoretical study of the multiplet structure observed by x-ray photoelectron spectroscopy. This correlated multiplet hole theory resolves the difficulties of earlier multiplet hole theory studies: It correctly determines the magnitude of the observed 2s and 3s (doublet) splittings and their intensity rations, and predicts the existence of new structure for the 3s binding energy splittings-structure which does not exist in one-electron theory and which has now been confirmed by Kowalczyk et al.",

author = "Bagus, {P. S.} and Freeman, {A. J.} and F. Sasaki",

note = "Funding Information: Work supported by the U. S. Air Force Office of Scientific Research, by the U. S. Atomic Energy Commission, and by the National Science Foundation. Copyright: Copyright 2015 Elsevier B.V., All rights reserved.",

year = "1973",

doi = "10.1103/PhysRevLett.30.850",

language = "English (US)",

volume = "30",

pages = "850--853",

journal = "Physical review letters",

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T1 - Prediction of new multiplet structure in photoemission experiments

AU - Bagus, P. S.

AU - Freeman, A. J.

AU - Sasaki, F.

N1 - Funding Information: Work supported by the U. S. Air Force Office of Scientific Research, by the U. S. Atomic Energy Commission, and by the National Science Foundation. Copyright: Copyright 2015 Elsevier B.V., All rights reserved.

PY - 1973

Y1 - 1973

N2 - Correlation effects are included in a detailed theoretical study of the multiplet structure observed by x-ray photoelectron spectroscopy. This correlated multiplet hole theory resolves the difficulties of earlier multiplet hole theory studies: It correctly determines the magnitude of the observed 2s and 3s (doublet) splittings and their intensity rations, and predicts the existence of new structure for the 3s binding energy splittings-structure which does not exist in one-electron theory and which has now been confirmed by Kowalczyk et al.

AB - Correlation effects are included in a detailed theoretical study of the multiplet structure observed by x-ray photoelectron spectroscopy. This correlated multiplet hole theory resolves the difficulties of earlier multiplet hole theory studies: It correctly determines the magnitude of the observed 2s and 3s (doublet) splittings and their intensity rations, and predicts the existence of new structure for the 3s binding energy splittings-structure which does not exist in one-electron theory and which has now been confirmed by Kowalczyk et al.

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Prediction of new multiplet structure in photoemission experiments

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