Resilience of monolayer MoS2 memtransistor under heavy ion irradiation

Christopher M. Smyth*, John M. Cain, Eric J. Lang, Ping Lu, Xiaodong Yan, Stephanie E. Liu, Jiangtan Yuan, Matthew P. Bland, Nathan J. Madden, Taisuke Ohta, Vinod K. Sangwan, Mark C. Hersam, Khalid Hattar, Stanley S. Chou, Tzu Ming Lu

*Corresponding author for this work

Research output: Contribution to journalArticlepeer-review

Abstract

Due to its unique gate-tunable non-volatility, the memtransistor is a promising component for low-energy neuromorphic computing. The grain boundary- and point defect-enabled resistive switching in MoS2 memtransistors suggests an inherent ionizing radiation tolerance. However, the memtransistor resilience under heavy ion irradiation has not yet been investigated. In this work, polycrystalline, monolayer MoS2 films, and memtransistors are irradiated with 48 keV Au. Fluence-dependent effects on the MoS2 lattice structure, chemical states, and memtransistor performance metrics are elucidated. When the Au fluence remains below 1013 cm−2, the memtransistor functionalities are preserved. When the Au fluence exceeds 1014 cm−2, the MoS2 is amorphized and memtransistor functionalities are lost. According to Raman spectroscopy and transmission electron microscopy, the MoS2 defect concentration increases with increasing Au fluence. X-ray photoelectron spectroscopy substantiates a significant S:Mo ratio reduction with increasing Au fluence. This work suggests that MoS2 memtransistors possess sufficient heavy ion resilience for few-year space missions. Graphical abstract: [Figure not available: see fulltext.]

Original languageEnglish (US)
Pages (from-to)2723-2737
Number of pages15
JournalJournal of Materials Research
Volume37
Issue number17
DOIs
StatePublished - Sep 14 2022

Keywords

  • Defect
  • Ionizing radiation
  • Memtransistor
  • MoS
  • Radiation tolerance

ASJC Scopus subject areas

  • Materials Science(all)
  • Condensed Matter Physics
  • Mechanics of Materials
  • Mechanical Engineering

Fingerprint

Dive into the research topics of 'Resilience of monolayer MoS2 memtransistor under heavy ion irradiation'. Together they form a unique fingerprint.

Cite this