The use of intense-field ionization in time-resolved measurements

Tamar Seideman; M. Yu Ivanov; P. B. Corkum

doi:10.1016/0009-2614(96)00145-5

The use of intense-field ionization in time-resolved measurements

Tamar Seideman^*, M. Yu Ivanov, P. B. Corkum

^*Corresponding author for this work

Chemistry

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30 Scopus citations

Abstract

We show that intense radiation introduces a length-scale in molecules which translates into a dramatic enhancement of the rate of multiple ionization of molecules at characteristic internuclear separations. This feature is common to a wide range of systems and is insensitive to variations in frequency and intensity. The electronic properties responsible for this effect are explored. We propose the use of the sensitivity of intense-field ionization to the molecular configuration as a probe in time-resolved studies of dissociative dynamics.

Original language	English (US)
Pages (from-to)	181-188
Number of pages	8
Journal	Chemical Physics Letters
Volume	252
Issue number	3-4
DOIs	https://doi.org/10.1016/0009-2614(96)00145-5
State	Published - Apr 12 1996

ASJC Scopus subject areas

General Physics and Astronomy
Physical and Theoretical Chemistry

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10.1016/0009-2614(96)00145-5

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abstract = "We show that intense radiation introduces a length-scale in molecules which translates into a dramatic enhancement of the rate of multiple ionization of molecules at characteristic internuclear separations. This feature is common to a wide range of systems and is insensitive to variations in frequency and intensity. The electronic properties responsible for this effect are explored. We propose the use of the sensitivity of intense-field ionization to the molecular configuration as a probe in time-resolved studies of dissociative dynamics.",

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AU - Ivanov, M. Yu

AU - Corkum, P. B.

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N2 - We show that intense radiation introduces a length-scale in molecules which translates into a dramatic enhancement of the rate of multiple ionization of molecules at characteristic internuclear separations. This feature is common to a wide range of systems and is insensitive to variations in frequency and intensity. The electronic properties responsible for this effect are explored. We propose the use of the sensitivity of intense-field ionization to the molecular configuration as a probe in time-resolved studies of dissociative dynamics.

AB - We show that intense radiation introduces a length-scale in molecules which translates into a dramatic enhancement of the rate of multiple ionization of molecules at characteristic internuclear separations. This feature is common to a wide range of systems and is insensitive to variations in frequency and intensity. The electronic properties responsible for this effect are explored. We propose the use of the sensitivity of intense-field ionization to the molecular configuration as a probe in time-resolved studies of dissociative dynamics.

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The use of intense-field ionization in time-resolved measurements

Abstract

ASJC Scopus subject areas

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