Abstract
The accuracy of the approach of computing the ionization matrix elements through comparison of time-resolved photoelectron imaging (PEI) observables computed with this and with a more accurate approach was examined. As such, the time-dependent DFT (TDDFT) approach, a method of increasing popularity whose advantages over KS were illustrated in a variety of recent electronic structure applications was used. This paper takes advantage of the computed ionization matrix elements to explore several interesting features of time-resolved PEI that were not discussed before and others that need attention.
Original language | English (US) |
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Pages (from-to) | 1172-1180 |
Number of pages | 9 |
Journal | Journal of Chemical Physics |
Volume | 120 |
Issue number | 3 |
DOIs | |
State | Published - Jan 15 2004 |
ASJC Scopus subject areas
- General Physics and Astronomy
- Physical and Theoretical Chemistry