Theory of Time-Resolved Photoelectron Imaging: Nonperturbative Calculation for an Internally Converting Polyatomic Molecule

Yoshi Ichi Suzuki; Mauro Stener; Tamar Seideman

doi:10.1103/PhysRevLett.89.233002

Theory of Time-Resolved Photoelectron Imaging: Nonperturbative Calculation for an Internally Converting Polyatomic Molecule

Yoshi Ichi Suzuki, Mauro Stener, Tamar Seideman^*

^*Corresponding author for this work

Chemistry

Research output: Contribution to journal › Article › peer-review

21 Scopus citations

Abstract

We present the first calculation of time-resolved photoelectron angular distributions for a polyatomic system. Our method takes rotations into exact account, treats the laser field nonperturbatively, and computes the electronic dynamics from first principles. Our results point to the information content of time-resolved photoelectron imaging observables and illustrate the role played by the field intensity.

Original language	English (US)
Journal	Physical review letters
Volume	89
Issue number	23
DOIs	https://doi.org/10.1103/PhysRevLett.89.233002
State	Published - 2002

ASJC Scopus subject areas

General Physics and Astronomy

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10.1103/PhysRevLett.89.233002

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title = "Theory of Time-Resolved Photoelectron Imaging: Nonperturbative Calculation for an Internally Converting Polyatomic Molecule",

abstract = "We present the first calculation of time-resolved photoelectron angular distributions for a polyatomic system. Our method takes rotations into exact account, treats the laser field nonperturbatively, and computes the electronic dynamics from first principles. Our results point to the information content of time-resolved photoelectron imaging observables and illustrate the role played by the field intensity.",

author = "Suzuki, {Yoshi Ichi} and Mauro Stener and Tamar Seideman",

year = "2002",

doi = "10.1103/PhysRevLett.89.233002",

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AU - Seideman, Tamar

PY - 2002

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AB - We present the first calculation of time-resolved photoelectron angular distributions for a polyatomic system. Our method takes rotations into exact account, treats the laser field nonperturbatively, and computes the electronic dynamics from first principles. Our results point to the information content of time-resolved photoelectron imaging observables and illustrate the role played by the field intensity.

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Theory of Time-Resolved Photoelectron Imaging: Nonperturbative Calculation for an Internally Converting Polyatomic Molecule

Abstract

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