TY - JOUR
T1 - Theory predicts 2D chiral polaritons based on achiral Fabry–Pérot cavities using apparent circular dichroism
AU - Salij, Andrew H.
AU - Goldsmith, Randall H.
AU - Tempelaar, Roel
N1 - Publisher Copyright:
© 2024, The Author(s).
PY - 2024/12
Y1 - 2024/12
N2 - Realizing polariton states with high levels of chirality offers exciting prospects for quantum information, sensing, and lasing applications. Such chirality must emanate from either the involved optical resonators or the quantum emitters. Here, we theoretically demonstrate a rare opportunity for realizing polaritons with so-called 2D chirality by strong coupling of the optical modes of (high finesse) achiral Fabry–Pérot cavities with samples exhibiting “apparent circular dichroism” (ACD). ACD is a phenomenon resulting from an interference between linear birefringence and dichroic interactions. By introducing a quantum electrodynamical theory of ACD, we identify the design rules based on which 2D chiral polaritons can be produced, and their chirality can be optimized.
AB - Realizing polariton states with high levels of chirality offers exciting prospects for quantum information, sensing, and lasing applications. Such chirality must emanate from either the involved optical resonators or the quantum emitters. Here, we theoretically demonstrate a rare opportunity for realizing polaritons with so-called 2D chirality by strong coupling of the optical modes of (high finesse) achiral Fabry–Pérot cavities with samples exhibiting “apparent circular dichroism” (ACD). ACD is a phenomenon resulting from an interference between linear birefringence and dichroic interactions. By introducing a quantum electrodynamical theory of ACD, we identify the design rules based on which 2D chiral polaritons can be produced, and their chirality can be optimized.
UR - http://www.scopus.com/inward/record.url?scp=85181531061&partnerID=8YFLogxK
UR - http://www.scopus.com/inward/citedby.url?scp=85181531061&partnerID=8YFLogxK
U2 - 10.1038/s41467-023-44523-1
DO - 10.1038/s41467-023-44523-1
M3 - Article
C2 - 38184645
AN - SCOPUS:85181531061
SN - 2041-1723
VL - 15
JO - Nature communications
JF - Nature communications
IS - 1
M1 - 340
ER -